Negative Entropy of Mixing for Vanadium-Platinum Solutions

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Negative entropy of mixing for vanadium-platinum solutions.

The phonon densities of states for pure vanadium and the solid solutions V-6.25% Ni, Pd, Pt were determined from inelastic neutron scattering measurements. The solute atoms caused a large stiffening of the phonons, resulting in large, negative vibrational entropies of mixing. For V-6.25%Pt, the negative vibrational entropy of mixing exceeds the conventional positive chemical entropy of mixing. ...

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ژورنال

عنوان ژورنال: Physical Review Letters

سال: 2004

ISSN: 0031-9007,1079-7114

DOI: 10.1103/physrevlett.93.185704